Segmental Relaxation in Poly(dimethylsiloxane)
Note: In lieu of an abstract, this is the article's first page.
*
In papers with more than one author, the asterisk indicates the name of the author to whom inquiries about the paper should be addressed.
Cited By
This article is cited by 65 publications.
- Louis Poon, Jacob R. Hum, Richard G. Weiss. Ion-Transport Properties of Polydimethylsiloxane-Based Ionomers with Amidinium or Imidazolinium Alkyldithiocarbamate Pendant Groups in Low Dielectric Solvents or as Neat Liquids. The Journal of Physical Chemistry B 2022, 126 (49) , 10481-10489. https://doi.org/10.1021/acs.jpcb.2c05431
- Pei Bai, Mingchao Ma, Li Sui, Yunlong Guo. Nanoconfinement Controls Mechanical Properties of Elastomeric Thin Films. The Journal of Physical Chemistry Letters 2021, 12 (33) , 8072-8079. https://doi.org/10.1021/acs.jpclett.1c01921
- Manjesh K. Singh, Minghan Hu, Yu Cang, Hsiao-Ping Hsu, Heloise Therien-Aubin, Kaloian Koynov, George Fytas, Katharina Landfester, Kurt Kremer. Glass Transition of Disentangled and Entangled Polymer Melts: Single-Chain-Nanoparticles Approach. Macromolecules 2020, 53 (17) , 7312-7321. https://doi.org/10.1021/acs.macromol.0c00550
- Agnieszka Talik, Magdalena Tarnacka, Andrzej Dzienia, Ewa Kaminska, Kamil Kaminski, Marian Paluch. High-Pressure Studies on the Chain and Segmental Dynamics of a Series of Poly(propylene glycol) Derivatives. Macromolecules 2019, 52 (15) , 5658-5669. https://doi.org/10.1021/acs.macromol.9b00692
- Jialong Shen, Erol Yildirim, Shanshan Li, Yavuz Caydamli, Melissa A. Pasquinelli, Alan E. Tonelli. Role of Local Polymer Conformations on the Diverging Glass Transition Temperatures and Dynamic Fragilities of Isotactic-, Syndiotactic-, and Atactic-Poly(methyl methacrylate)s. Macromolecules 2019, 52 (10) , 3897-3908. https://doi.org/10.1021/acs.macromol.9b00434
- Magdalena Tarnacka, Agnieszka Talik, Ewa Kamińska, Monika Geppert-Rybczyńska, Kamil Kaminski, Marian Paluch. The Impact of Molecular Weight on the Behavior of Poly(propylene glycol) Derivatives Confined within Alumina Templates. Macromolecules 2019, 52 (9) , 3516-3529. https://doi.org/10.1021/acs.macromol.9b00209
- Valeria Arrighi, Simona Gagliardi, Fabio Ganazzoli, Julia S. Higgins, Giuseppina Raffaini, Jeerachada Tanchawanich, Jenny Taylor, Mark T. F. Telling. Effect of Chain Length and Topological Constraints on Segmental Relaxation in Cyclic PDMS. Macromolecules 2018, 51 (18) , 7209-7223. https://doi.org/10.1021/acs.macromol.8b00397
- Junliang Zhang, Robert Deubler, Matthias Hartlieb, Liam Martin, Joji Tanaka, Elena Patyukova, Paul D. Topham, Felix H. Schacher, and Sébastien Perrier . Evolution of Microphase Separation with Variations of Segments of Sequence-Controlled Multiblock Copolymers. Macromolecules 2017, 50 (18) , 7380-7387. https://doi.org/10.1021/acs.macromol.7b01831
- Shadid Askar, Lingqiao Li, and John M. Torkelson . Polystyrene-Grafted Silica Nanoparticles: Investigating the Molecular Weight Dependence of Glass Transition and Fragility Behavior. Macromolecules 2017, 50 (4) , 1589-1598. https://doi.org/10.1021/acs.macromol.7b00079
- Lanhe Zhang, Ravinder Elupula, Scott M. Grayson, and John M. Torkelson . Suppression of the Fragility-Confinement Effect via Low Molecular Weight Cyclic or Ring Polymer Topology. Macromolecules 2017, 50 (3) , 1147-1154. https://doi.org/10.1021/acs.macromol.6b02280
- Shi-Jie Xie and Kenneth S. Schweizer . Nonuniversal Coupling of Cage Scale Hopping and Collective Elastic Distortion as the Origin of Dynamic Fragility Diversity in Glass-Forming Polymer Liquids. Macromolecules 2016, 49 (24) , 9655-9664. https://doi.org/10.1021/acs.macromol.6b02272
- Lanhe Zhang, John A. Marsiglio, Tian Lan, and John M. Torkelson . Dramatic Tunability of the Glass Transition Temperature and Fragility of Low Molecular Weight Polystyrene by Initiator Fragments Located at Chain Ends. Macromolecules 2016, 49 (6) , 2387-2398. https://doi.org/10.1021/acs.macromol.5b02704
- K. Kaminski, W. K. Kipnusu, K. Adrjanowicz, E. U. Mapesa, C. Iacob, M. Jasiurkowska, P. Wlodarczyk, K. Grzybowska, M. Paluch, and F. Kremer . Comparative Study on the Molecular Dynamics of a Series of Polypropylene Glycols. Macromolecules 2013, 46 (5) , 1973-1980. https://doi.org/10.1021/ma302611x
- A. Bormuth, P. Henritzi, and M. Vogel. Chain-Length Dependence of the Segmental Relaxation in Polymer Melts: Molecular Dynamics Simulation Studies on Poly(propylene oxide). Macromolecules 2010, 43 (21) , 8985-8992. https://doi.org/10.1021/ma101721d
- Yohei Miwa, Shigetaka Shimada, Osamu Urakawa and Shogo Nobukawa . Origin of High Segmental Mobility at Chain Ends of Polystyrene. Macromolecules 2010, 43 (17) , 7192-7199. https://doi.org/10.1021/ma1013644
- Christine Gerstl, Gerald J. Schneider, Wim Pyckhout-Hintzen, Jürgen Allgaier, Dieter Richter, Angel Alegría and Juan Colmenero . Segmental and Normal Mode Relaxation of Poly(alkylene oxide)s Studied by Dielectric Spectroscopy and Rheology. Macromolecules 2010, 43 (11) , 4968-4977. https://doi.org/10.1021/ma100384j
- J. Hintermeyer, A. Herrmann, R. Kahlau, C. Goiceanu and E. A. Rössler. Molecular Weight Dependence of Glassy Dynamics in Linear Polymers Revisited. Macromolecules 2008, 41 (23) , 9335-9344. https://doi.org/10.1021/ma8016794
- C. M. Roland and, R. Casalini. Dynamics of Poly(cyclohexyl methacrylate): Neat and in Blends with Poly(α-methylstyrene). Macromolecules 2007, 40 (10) , 3631-3639. https://doi.org/10.1021/ma0702849
- Shanfeng Wang,, Lichun Lu, and, Michael J. Yaszemski. Bone-Tissue-Engineering Material Poly(propylene fumarate): Correlation between Molecular Weight, Chain Dimensions, and Physical Properties. Biomacromolecules 2006, 7 (6) , 1976-1982. https://doi.org/10.1021/bm060096a
- Shanfeng Wang,, Lichun Lu,, James A. Gruetzmacher,, Bradford L. Currier, and, Michael J. Yaszemski. A Biodegradable and Cross-Linkable Multiblock Copolymer Consisting of Poly(propylene fumarate) and Poly(ε-caprolactone): Synthesis, Characterization, and Physical Properties. Macromolecules 2005, 38 (17) , 7358-7370. https://doi.org/10.1021/ma050884c
- Yohei Miwa,, Katsuhiro Yamamoto,, Masato Sakaguchi,, Masahiro Sakai,, Seiji Makita, and, Shigetaka Shimada. Direct Detection of High Mobility around Chain Ends of Poly(methyl methacrylate) by the Spin-Labeling. Macromolecules 2005, 38 (3) , 832-838. https://doi.org/10.1021/ma048287y
- Yifu Ding,, V. N. Novikov, and, A. P. Sokolov, , R. Casalini and, C. M. Roland. Observation of Chain Dynamics in Depolarized Light Scattering Spectra of Polymers. Macromolecules 2004, 37 (24) , 9273-9278. https://doi.org/10.1021/ma048718c
- Yifu Ding,, V. N. Novikov, and, A. P. Sokolov, , A. Cailliaux,, C. Dalle-Ferrier, and, C. Alba-Simionesco, , B. Frick. Influence of Molecular Weight on Fast Dynamics and Fragility of Polymers. Macromolecules 2004, 37 (24) , 9264-9272. https://doi.org/10.1021/ma0492420
- C. M. Roland,, R. Casalini,, P. Santangelo,, M. Sekula,, J. Ziolo, and, M. Paluch. Chemical Structure and Local Segmental Dynamics in 1,2-Polybutadiene. Macromolecules 2003, 36 (13) , 4954-4959. https://doi.org/10.1021/ma034416j
- C. M. Roland and, R. Casalini. Temperature and Volume Effects on Local Segmental Relaxation in Poly(vinyl acetate). Macromolecules 2003, 36 (4) , 1361-1367. https://doi.org/10.1021/ma025791z
- M. J. Schroeder, , C. M. Roland. Segmental Relaxation in End-Linked Poly(dimethylsiloxane) Networks. Macromolecules 2002, 35 (7) , 2676-2681. https://doi.org/10.1021/ma011678h
- P. G. Santangelo and, C. M. Roland, , Taihyun Chang and, Donghyun Cho, , Jacques Roovers. Dynamics near the Glass Temperature of Low Molecular Weight Cyclic Polystyrene. Macromolecules 2001, 34 (26) , 9002-9005. https://doi.org/10.1021/ma011069+
- Sheila N. Daniel,, Emily D. Niemeyer, and, Frank V. Bright. Evidence for Chain Length Dependent Local Ordering Surrounding Perylene Dissolved in Poly(ethylene glycol). Macromolecules 1999, 32 (24) , 8084-8088. https://doi.org/10.1021/ma990674y
- Apostolos K. Rizos, , K. L. Ngai. Local Segmental Dynamics of Low Molecular Weight Polystyrene: New Results and Interpretation. Macromolecules 1998, 31 (18) , 6217-6225. https://doi.org/10.1021/ma980613k
- P. G. Santangelo and, C. M. Roland. Molecular Weight Dependence of Fragility in Polystyrene. Macromolecules 1998, 31 (14) , 4581-4585. https://doi.org/10.1021/ma971823k
- Emily D. Niemeyer and, Frank V. Bright. Effects of CO2 Sorption on the Rotational Reorientation Dynamics of a Model Solute Dissolved in Molten Poly(dimethylsiloxane). Macromolecules 1998, 31 (1) , 77-85. https://doi.org/10.1021/ma970335+
- K. L. Ngai and, C. M. Roland. Short-Time Relaxational Dynamics of the “Strong” Glass-Former Methanol. The Journal of Physical Chemistry B 1997, 101 (22) , 4437-4441. https://doi.org/10.1021/jp963352u
- Daisuke Kawaguchi, Ayano Higasayama, Yudai Ogata, Taizo Kabe, Yushu Matsushita, Keiji Tanaka. Crystalline structure, molecular motion and photocarrier formation in thin films of monodisperse poly(3-hexylthiophene) with various molecular weights. Polymer Journal 2023, 55 (4) , 497-505. https://doi.org/10.1038/s41428-022-00713-0
- Valeria Arrighi, Julia S. Higgins. Local Effects of Ring Topology Observed in Polymer Conformation and Dynamics by Neutron Scattering—A Review. Polymers 2020, 12 (9) , 1884. https://doi.org/10.3390/polym12091884
- Angelika Wrzesińska, Izabela Bobowska, Paulina Maczugowska, Joanna Małolepsza, Katarzyna M. Błażewska, Aleksandra Wypych-Puszkarz. Effect of Metal-Ligand Coordination Complexes on Molecular Dynamics and Structure of Cross-Linked Poly(dimethylosiloxane). Polymers 2020, 12 (8) , 1680. https://doi.org/10.3390/polym12081680
- Shaoyong Huang, Hongfei Li, Shichun Jiang. Crystal structure and unique lamellar thickening for poly(l-lactide) induced by high pressure. Polymer 2019, 175 , 81-86. https://doi.org/10.1016/j.polymer.2019.05.020
- A. Roggero, E. Dantras, T. Paulmier, C. Tonon, S. Lewandowski, S. Dagras, D. Payan. Dynamic glass transition of filled polysiloxane upon electron irradiation. Journal of Non-Crystalline Solids 2017, 455 , 17-23. https://doi.org/10.1016/j.jnoncrysol.2016.10.025
- C. Ghisleri, M. A. C. Potenza, L. Ravagnan, A. Bellacicca, P. Milani. A simple scanning spectrometer based on a stretchable elastomeric reflective grating. Applied Physics Letters 2014, 104 (6) https://doi.org/10.1063/1.4865427
- Yan Jin, MingShi Song, GuiXian Hu, DaMing Wu. Correlation of cooperatively localized rearrangement on the “fluidized domain” in glass substances (or polymers) to their fragility III: Theory of dynamic fragility at isochoric state. Science China Physics, Mechanics and Astronomy 2011, 54 (3) , 420-436. https://doi.org/10.1007/s11433-010-4236-2
- K.L. Ngai. Glass-Forming Substances and Systems. 2011, 49-638. https://doi.org/10.1007/978-1-4419-7649-9_2
- Evgeny B. Stukalin, Jack F. Douglas, Karl F. Freed. Application of the entropy theory of glass formation to poly(α-olefins). The Journal of Chemical Physics 2009, 131 (11) https://doi.org/10.1063/1.3216109
- L. P. Singh, S. S. N. Murthy. Study of secondary relaxation in disordered plastic crystals of isocyanocyclohexane, cyanocyclohexane, and 1-cyanoadamantane. The Journal of Chemical Physics 2008, 129 (9) https://doi.org/10.1063/1.2961036
- K. Kunal, M. Paluch, C. M. Roland, J. E. Puskas, Y. Chen, A. P. Sokolov. Polyisobutylene: A most unusual polymer. Journal of Polymer Science Part B: Polymer Physics 2008, 46 (13) , 1390-1399. https://doi.org/10.1002/polb.21473
- Klaus Schröter, Sven Reissig, Elke Hempel, Mario Beiner. From small molecules to polymers: Relaxation behavior of n-butyl methacrylate based systems. Journal of Non-Crystalline Solids 2007, 353 (41-43) , 3976-3983. https://doi.org/10.1016/j.jnoncrysol.2007.02.062
- J. Salud, D.O. López, S. Diez-Berart, M.A. Pérez-Jubindo, M.R. de la Fuente, M.A. Rute. Some insights into fragility as a function of thermodynamic parameters: From orientational to structural glass transitions. Chemical Physics Letters 2007, 446 (1-3) , 71-76. https://doi.org/10.1016/j.cplett.2007.08.052
- V.M. Gun’ko, M.V. Borysenko, P. Pissis, A. Spanoudaki, N. Shinyashiki, I.Y. Sulim, T.V. Kulik, B.B. Palyanytsya. Polydimethylsiloxane at the interfaces of fumed silica and zirconia/fumed silica. Applied Surface Science 2007, 253 (17) , 7143-7156. https://doi.org/10.1016/j.apsusc.2007.02.185
- A P Sokolov, V N Novikov, Y Ding. Why many polymers are so fragile. Journal of Physics: Condensed Matter 2007, 19 (20) , 205116. https://doi.org/10.1088/0953-8984/19/20/205116
- R. Casalini, C. M. Roland, S. Capaccioli. Effect of chain length on fragility and thermodynamic scaling of the local segmental dynamics in poly(methylmethacrylate). The Journal of Chemical Physics 2007, 126 (18) https://doi.org/10.1063/1.2728898
- Qian Qin, Gregory B. McKenna. Correlation between dynamic fragility and glass transition temperature for different classes of glass forming liquids. Journal of Non-Crystalline Solids 2006, 352 (28-29) , 2977-2985. https://doi.org/10.1016/j.jnoncrysol.2006.04.014
- Kenneth S. Schweizer, Erica J. Saltzman. Theory of dynamic barriers, activated hopping, and the glass transition in polymer melts. The Journal of Chemical Physics 2004, 121 (4) , 1984-2000. https://doi.org/10.1063/1.1756854
- C. G. Robertson, C. M. Roland. Local segmental relaxation in bidisperse polystyrenes. Journal of Polymer Science Part B: Polymer Physics 2004, 42 (13) , 2604-2611. https://doi.org/10.1002/polb.20127
- C. M. Roland, R. Casalini. Temperature dependence of local segmental motion in polystyrene and its variation with molecular weight. The Journal of Chemical Physics 2003, 119 (3) , 1838-1842. https://doi.org/10.1063/1.1581850
- C. M. Roland, P. G. Santangelo, C. G. Robertson, K. L. Ngai. Comment on “Direct determination of kinetic fragility indices of glassforming liquids by differential scanning calorimetry: Kinetic versus thermodynamic fragilities” [J. Chem. Phys. 117 , 10184 (2002)]. The Journal of Chemical Physics 2003, 118 (22) , 10351-10352. https://doi.org/10.1063/1.1571814
- M. Paluch, C. M. Roland, S. Pawlus. Temperature and pressure dependence of the α-relaxation in polymethylphenylsiloxane. The Journal of Chemical Physics 2002, 116 (24) , 10932-10937. https://doi.org/10.1063/1.1478767
- Robert F. Brady. Clean hulls without poisons: Devising and testing nontoxic marine coatings. Journal of Coatings Technology 2000, 72 (1) , 45-56. https://doi.org/10.1007/BF02698394
- C. M. Roland, P. G. Santangelo, D. J. Plazek, K. M. Bernatz. Creep of selenium near the glass temperature. The Journal of Chemical Physics 1999, 111 (20) , 9337-9342. https://doi.org/10.1063/1.479846
- Dino Ferri, Paolo Lomellini. Melt rheology of randomly branched polystyrenes. Journal of Rheology 1999, 43 (6) , 1355-1372. https://doi.org/10.1122/1.551048
- C. M. Roland, P. G. Santangelo, K. L. Ngai. The application of the energy landscape model to polymers. The Journal of Chemical Physics 1999, 111 (12) , 5593-5598. https://doi.org/10.1063/1.479861
- Christo Alexandrov Solunov. Cooperative molecular dynamics and strong/fragile behavior of polymers. European Polymer Journal 1999, 35 (8) , 1543-1556. https://doi.org/10.1016/S0014-3057(98)00226-2
- C. León, K. L. Ngai, C. M. Roland. Relationship between the primary and secondary dielectric relaxation processes in propylene glycol and its oligomers. The Journal of Chemical Physics 1999, 110 (23) , 11585-11591. https://doi.org/10.1063/1.478006
- Rodney J. Andrews, Eric A. Grulke. Glass Transition Temperatures of Polymers. 1999https://doi.org/10.1002/0471532053.bra039
- P. G. Santangelo, C. M. Roland. Test of the energy landscape interpretation of fragility in polymers. Physical Review B 1998, 58 (21) , 14121-14123. https://doi.org/10.1103/PhysRevB.58.14121
- P.G. Santangelo, K.L. Ngai, C.M. Roland. The coupling model approach to the terminal relaxation. Polymer 1998, 39 (3) , 681-687. https://doi.org/10.1016/S0032-3861(97)00315-7
- C.M. Roland, K.L. Ngai. Commentary on ‘Strong and fragile liquids - A brief critique’. Journal of Non-Crystalline Solids 1997, 212 (1) , 74-76. https://doi.org/10.1016/S0022-3093(96)00684-9
- C.M. Roland, K.L. Ngai, D.J. Plazek. The viscoelastic behaviour of networks. Computational and Theoretical Polymer Science 1997, 7 (3-4) , 133-137. https://doi.org/10.1016/S1089-3156(97)00016-0