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SWNT−MWNT Hybrid Filter Attains High Viral Removal and Bacterial Inactivation

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Department of Chemical and Environmental Engineering, Yale University, New Haven, Connecticut 06520-8286, United States
*Corresponding author. E-mail: [email protected]. Phone: +1 (203) 432-2789.
†Current address: Department of Civil and Environmental Engineering, University of Alberta, Edmonton, Alberta, Canada T6G 2W2
Cite this: Langmuir 2010, 26, 24, 19153–19158
Publication Date (Web):November 23, 2010
https://doi.org/10.1021/la103776y
Copyright © 2010 American Chemical Society
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    Abstract

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    We describe the concept and demonstrate the efficacy of a novel SWNT−MWNT hybrid filter for the removal and inactivation of microbial pathogens from water. The filter is composed of a thin SWNT layer (0.05 mg cm−2) on top of a thicker MWNT layer (0.27 mg cm−2) supported by a microporous support membrane. The SWNT−MWNT filter exhibits high log removal of several model viruses (MS2, PRD1, and T4 bacteriophages) by depth filtration, which predominantly takes place in the thicker and more uniform MWNT layer. The filter removes all bacteria by a sieving mechanism, with the top SWNT layer providing high levels of inactivation of model bacteria (Escherichia coli K12 and Staphylococcus epidermidis), as well as microbes from river water and treated wastewater effluent. The dual-layer SWNT−MWNT filter lays the framework for new possibilities in point-of-use water filtration.

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