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Polarized Plasmonic Enhancement by Au Nanostructures Probed through Raman Scattering of Suspended Graphene

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† Department of Physics, Freie Universität Berlin, 14195 Berlin, Germany
‡ Department of Physics, Imperial College London, London SW7 2AZ, U.K.
¶ § School of Computer Science and §Centre for Mesoscience and Nanotechnology, The University of Manchester, Manchester M13 9PL, U.K.
*E-mail: [email protected]
Cite this: Nano Lett. 2013, 13, 1, 301–308
Publication Date (Web):December 7, 2012
https://doi.org/10.1021/nl3041542
Copyright © 2012 American Chemical Society
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    Abstract

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    We characterize plasmonic enhancement in a hotspot between two Au nanodisks using Raman scattering of graphene. Single layer graphene is suspended across the dimer cavity and provides an ideal two-dimensional test material for the local near-field distribution. We detect a Raman enhancement of the order of 103 originating from the cavity. Spatially resolved Raman measurements reveal a near-field localization one order of magnitude smaller than the wavelength of the excitation, which can be turned off by rotating the polarization of the excitation. The suspended graphene is under tensile strain. The resulting phonon mode softening allows for a clear identification of the enhanced signal compared to unperturbed graphene.

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    Fabrication and structural characterization; optical characterization; simulations; AFM data on dimers before and after graphene deposition; microscope images of graphene flake; AFM data and graphene topography on different structure; 2D peak fits for PX; Raman line scan raw data for 638 nm excitation; laser spot profile; intensity drop for 532 nm excitation. This material is available free of charge via the Internet at http://pubs.acs.org.

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